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The present disclosure relates to a method for making a thermal interface material. A carbon nanotube array on a substrate is provided. The carbon nanotube array includes a plurality of carbon nanotubes substantially parallel to each other and substantially perpendicular to the substrate. The carbon

The present disclosure relates to a method for making a thermal interface material. A carbon nanotube array on a substrate is provided. The carbon nanotube array includes a plurality of carbon nanotubes substantially parallel to each other and substantially perpendicular to the substrate. The carbon nanotubes of the carbon nanotube array are slanted toward a central axis of the carbon nanotube array. A liquid matrix material is compounded with the carbon nanotube array. Additionally, the liquid matrix material is solidified.

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1. A method for making a thermal interface material, the method comprising: (a) providing a carbon nanotube array on a substrate, the carbon nanotube array comprising a plurality of carbon nanotubes substantially parallel to each other and substantially perpendicular to the substrate;(b) slanting th

1. A method for making a thermal interface material, the method comprising: (a) providing a carbon nanotube array on a substrate, the carbon nanotube array comprising a plurality of carbon nanotubes substantially parallel to each other and substantially perpendicular to the substrate;(b) slanting the carbon nanotubes of the carbon nanotube array toward a central axis of the carbon nanotube array to obtain slanted carbon nanotubes;(c) providing a liquid matrix material and compounding the liquid matrix material with the slanted carbon nanotubes of the carbon nanotube array; and(d) solidifying the liquid matrix material with the slanted carbon nanotubes to form a matrix. 2. The method of claim 1, wherein the carbon nanotube array has a first surface contacting with the substrate and a second surface opposite to the first surface. 3. The method of claim 2, wherein the carbon nanotube array is pressed by a mold to slant the carbon nanotubes toward the central axis of the carbon nanotube array. 4. The method of claim 3, wherein the mold is a hollow structure defined by sidewalls and has a first opening and a second opening opposite to the first opening, a size of the mold decreases along a direction from the second opening to the first opening. 5. The method of claim 4, wherein a shape of the second opening of the mold corresponds to a shape of the second surface of the carbon nanotube array; an area of the second opening is equal to or larger than an area of the second surface of the carbon nanotube array; and an area of the first opening is less than the area of the first surface of the carbon nanotube array. 6. The method of claim 4, wherein an inner surface of the mold is coated with a layer of mold releasing agent. 7. The method of claim 4, wherein the mold with the second opening opposite to the carbon nanotube array is covered on the carbon nanotube array from the first surface to the second surface, and the carbon nanotubes of the carbon nanotube array lean to the central axis of the carbon nanotube array under pressure of the sidewalls. 8. The method of claim 3, wherein the mold comprises a square frame with four sides joined end to end, and four isosceles trapezoid plates; a longer side of each isosceles trapezoid plate is fixed on the corresponding side of the square frame and rotatable around the longer side. 9. The method of claim 8, wherein a shape of the carbon nanotube array is square, and the mold is located around a square carbon nanotube array to press the carbon nanotube array by folding the four isosceles trapezoid plates. 10. The method of claim 1, wherein the liquid matrix material is a liquid phase change polymer, and the carbon nanotube array is immersed in the liquid phase change polymer. 11. The method of claim 1, wherein the liquid matrix material is a liquid phase change polymer or a low melting point metallic material, and the liquid matrix material is injected into the carbon nanotube array. 12. The method of claim 1, wherein the liquid matrix material is a low melting point metallic material, and the low melting point metallic material is plated into the carbon nanotube array. 13. The method of claim 12, wherein the low melting point metallic material is used as an anode, the carbon nanotube array is used as a cathode, and the mold is made of insulative material. 14. The method of claim 1, wherein the liquid matrix material is solidified by cooling, heating or adding an initiator. 15. The method of claim 1, further comprising a step (e) of removing the mold and the substrate. 16. The method of claim 15, wherein step (e) is executed by mechanical polishing, chemical etching or tearing directly. 17. A method for making a thermal interface material, the method comprising: (a) providing a carbon nanotube array comprising a plurality of carbon nanotubes on a substrate, the carbon nanotubes being substantially parallel to each other and substantially perpendicular to the substrate, the carbon nanotubes array having a central axis substantially parallel to each of the carbon nanotubes, the carbon nanotubes comprising a bottom end adjacent to the substrate and a top end away from the substrate;(b) slanting the carbon nanotubes of the carbon nanotube array toward the central axis of the carbon nanotubes array to obtain slanted carbon nanotubes, the top end of the slanted carbon nanotubes being closer to the central axis than the bottom end of the slanted carbon nanotubes;(c) introducing a liquid matrix material into the slanted carbon nanotubes of the carbon nanotube array; and(d) solidifying the liquid matrix material with the slanted carbon nanotubes to form a matrix. 18. The method of claim 17, further comprising slicing the thermal interface material to make the bottom ends and top ends of the nanotubes exposed from surfaces of the matrix. 19. The method of claim 17, further comprising etching the matrix to make the bottom ends and top ends of the nanotubes exposed from surfaces of the matrix. 20. A method for making a thermal interface material, the method comprising: (a) providing a carbon nanotube array formed on a substrate, the carbon nanotube array comprises a plurality of carbon nanotubes substantially parallel to each other and substantially perpendicular to the substrate;(b) slanting the carbon nanotubes of the carbon nanotube array toward the central axis of the carbon nanotube array to obtain slanted carbon nanotubes; and(c) introducing a matrix to compound with the slanted carbon nanotubes of the carbon nanotube array.