The invention relates to a process for improving the flavor of roasted Robusta and Arabica quality coffee and is characterized by modifying roasted coffee flavor precursors in aqueous extracts of green coffee beans.
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1. A method for preparing Robusta or Arabica quality coffee beans having improved coffee flavor, said method comprising: (1) extracting dry or pre-moistened Robusta or Arabica quality green coffee beans with an aqueous solution at about 60° C. to about 100° C. for about 2 to about 4 hours to obtain
1. A method for preparing Robusta or Arabica quality coffee beans having improved coffee flavor, said method comprising: (1) extracting dry or pre-moistened Robusta or Arabica quality green coffee beans with an aqueous solution at about 60° C. to about 100° C. for about 2 to about 4 hours to obtain (i) an aqueous extract containing water-soluble flavor precursors at about 4 to about 40 weight percent soluble solids, and (ii) extracted wet coffee beans having contacted surface water;(2) separating the aqueous extract and the extracted wet coffee beans having contacted surface water;(3) treating the separated aqueous extract to modify the water-soluble flavor precursors to obtain modified water-soluble flavor precursors, wherein the modified water-soluble flavor precursors are contained in the treated separated aqueous extract or are soluble solids obtained from the treated separated aqueous extract, wherein the treating is selected from one of heating the separated aqueous extract to hydrolyze water-soluble flavor precursors to organic acids, reducing levels of coumaryltryptophan and caffeoyltryptophan in the separated aqueous extract by contacting the separated aqueous extract with a hydrophobic or cation exchange resin, and treating the separated aqueous extract with a microorganism to reduce levels of caffeoylquinic acid and feruloylquinic acid in the separated extract;(4) combining the modified water-soluble flavor precursors with the separated extracted wet coffee beans having contacted surface water before drying to provide flavor-enhanced coffee beans; and(5) drying the flavor-enhanced coffee beans to obtain the Robusta or Arabica quality coffee beans having improved coffee flavor,wherein the aqueous solution used in step (1) is treated extract having modified water soluble flavor precursors which are used to extract water soluble flavor precursors from the green coffee beans. 2. The method of claim 1, and wherein the treating in step (3) comprises heating the separated aqueous extract at an elevated temperature and for a time sufficient to reduce the pH of the separated aqueous extract by about 0.2 to about 2 pH units and to form the modified water-soluble precursors. 3. The method of claim 2, wherein the green coffee beans are Arabica quality and wherein the elevated temperature is about 170 to about 250° C., the time is about 10 to about 360 sec., and the pH is reduced by about 0.5 to about 2 pH units. 4. The method of claim 2, wherein the green coffee beans are Arabica quality and wherein the elevated temperature is about 50 to about 90° C., the time is about 2 to about 60 hours, and the pH is reduced by about 0.5 to about 2 pH units. 5. The method of claim 3, wherein the elevated temperature is about 190 to about 230° C. and the pH is reduced by about 1 to about 2 pH units. 6. The method of claim 2, wherein the green coffee beans are Robusta quality and wherein the elevated temperature is about 170 to about 250° C., the time is about 10 to about 360 sec., and the pH is reduced by about 0.2 to about 1.2 pH units. 7. The method of claim 6, wherein the elevated temperature is about 190 to about 230° C. and the pH is reduced by about 0.4 to about 0.9 pH units. 8. The method of claim 2, wherein the aqueous solution used in step (1) includes a portion of the separated aqueous extract which has been treated to modify the water-soluble flavor precursors from step (3) which is recycled to step (1). 9. The method of claim 1, and wherein the treating in step (3) comprises reducing levels of coumaryltryptophan and caffeoyltryptophan in the separated aqueous extract by contacting the separated aqueous extract with about 2 to about 5 weight percent of the hydrophobic or cation exchange resin at about 5 to 60° C. for about 5 to about 30 minutes and then removing the hydrophobic or cation exchange resin to form the modified water-soluble precursors. 10. The method of claim 9, wherein the resin is polyvinylpyrrolidone and wherein the levels of coumaryltryptophan and caffeoyltryptophan in the coffee beans with improved coffee flavor are reduced by at least about 50 weight percent. 11. The method of claim 9, wherein the resin is polyvinylpyrrolidone and wherein the levels of coumaryltryptophan and caffeoyltryptophan in the coffee beans with improved coffee flavor are reduced by at least about 80 weight percent. 12. The method of claim 10, wherein the separated aqueous extract is contacted with the resin in step (3) for 2 to 5 times. 13. The method of claim 1, and wherein the treating in step (3) comprises treating the separated aqueous extract with the microorganism for about 12 to 120 hours to reduce levels of caffoylquinic acid and feruloylquinic acid in the separated aqueous extract and then removing the microorganism to form the modified water-soluble precursors. 14. The method of claim 13, wherein the microorganism is Rhodotorula mucilaginosa. 15. The method of claim 13, further comprising a step of adjusting sucrose level, pH value, or both sucrose level and pH value of the modified water-soluble flavor precursors to their corresponding level or value in the separated aqueous extract from step (1), wherein the adjustment is carried out before step (4). 16. The method of claim 14, further comprising a step of adjusting sucrose level, pH value, or both sucrose level and pH value of the modified water-soluble flavor precursors to their corresponding level or value in the separated aqueous extract from step (1), wherein the adjustment is carried out before step (4). 17. The method of claim 15, wherein the levels of caffoylquinic acid and feruloylquinic acid in the separated aqueous extract are each reduced by at least about 95 percent by weight. 18. The method of claim 16, wherein the levels of caffoylquinic acid and feruloylquinic acid in the separated aqueous extract are each reduced by at least about 95 percent by weight. 19. The method of claim 1, wherein pre-moistened Robusta or Arabica quality green coffee beans having a moisture content of about 50 to 60 weight percent are used in step (1). 20. The method of claim 9, wherein pre-moistened Robusta or Arabica quality green coffee beans having a moisture content of about 50 to 60 weight percent are used in step (1). 21. The method of claim 13, wherein pre-moistened Robusta or Arabica quality green coffee beans having a moisture content of about 50 to 60 weight percent are used in step (1). 22. Robusta or Arabica quality coffee beans having improved coffee flavor, said coffee beans being prepared by a method comprising: (1) extracting dry or pre-moistened Robusta or Arabica quality green coffee beans with an aqueous solution at about 60° C. to about 100° C. for about 2 to about 4 hours to obtain (i) an aqueous extract containing water-soluble flavor precursors at about 4 to about 40 weight percent soluble solids, and (ii) extracted wet coffee beans;(2) separating the aqueous extract and the extracted wet coffee beans;(3) treating the separated aqueous extract to modify the water-soluble flavor precursors to obtain modified water-soluble flavor precursors, wherein the modified water-soluble flavor precursors are contained in the treated separated aqueous extract or are soluble solids obtained from the treated separated aqueous extract, wherein the treating is selected from one of heating the separated aqueous extract to hydrolyze water-soluble flavor precursors to organic acids, reducing levels of coumaryltryptophan and caffeoyltryptophan in the separated aqueous extract by contacting the separated aqueous extract with a hydrophobic or cation exchange resin, and treating the separated aqueous extract with a microorganism to reduce levels of caffeoylquinic acid and feruloylquinic acid in the separated extract;(4) combining the modified water-soluble flavor precursors with the separated extracted wet coffee beans before drying to provide flavor-enhanced coffee beans; and(5) drying the flavor-enhanced coffee beans to obtain the Robusta or Arabica quality coffee beans having improved coffee flavor and wherein the aqueous solution used in step (1) is treated extract having modified water soluble flavor precursors which are used to extract water soluble flavor precursors from the green coffee beans. 23. The Robusta or Arabica quality coffee beans of claim 22, wherein the Robusta or Arabica quality coffee beans having improved coffee flavor of step (5) are roasted. 24. The Robusta or Arabica quality coffee beans of claim 22, wherein the coffee beans are of Robusta quality, wherein the coffee beans have a reduced pH of 4.8 to 5.2, a reduced sucrose content of less than about 2.0 g/100 g coffee beans and an increased total acid content of more than about 0.2 mmol/kg coffee beans. 25. The Robusta or Arabica quality coffee beans of claim 23, wherein the coffee beans are of Robusta quality, wherein the roasted coffee beans have a reduced vinyl-guiacol content of less than about 200 mg/kg roasted coffee beans and a reduced ethyl-pyrazine content of less than about 15 mg/kg roasted coffee beans. 26. The Robusta or Arabica quality coffee beans of claim 22, wherein the coffee green beans are of Arabica quality, wherein the coffee beans have a reduced pH of 4.5 to 5.0, a reduced sucrose content of less than about 3.5 g/100 g coffee beans and an increased total acid content of more than about 1.0 mmol/kg coffee beans. 27. The Robusta or Arabica quality coffee beans of claim 23, wherein the coffee beans are of Arabica quality, wherein the roasted coffee beans have a reduced vinyl-guiacol content of less than about 70 mg/kg roasted coffee beans and a reduced ethyl-pyrazine content of less than about 5 mg/kg roasted coffee beans. 28. The Robusta or Arabica quality coffee beans of claim 22, wherein the coffee beans are of Robusta quality, wherein the coffee beans have a reduced coumaryltryptophan content of less than about 0.05 g/kg coffee beans and a reduced caffeoyltryptophan content of less then about 1.0 g/kg coffee beans. 29. The Robusta or Arabica quality coffee beans of claim 23, wherein the coffee beans are of Robusta quality, wherein the roasted beans have a reduced coumaryltryptophan content of less than about 0.05 g/kg roasted coffee beans and a reduced caffeoyltryptophan content of less then about 1.0 g/kg roasted coffee beans, and a reduced 3-methylindol content of less than about 1.0 mg/kg roasted coffee beans. 30. The Robusta or Arabica quality coffee beans of claim 22, wherein the coffee beans are of Robusta quality, wherein the coffee beans have a reduced caffoylquinic acid content of less than about 350 mg/kg coffee beans, a reduced feruloylquinic acid content of less than about 450 mg/kg coffee beans, and a reduced caffeoyltryptophan content of less than about 1.0 g/kg coffee beans. 31. The Robusta or Arabica quality coffee beans of claim 23, wherein the coffee beans are of Robusta quality, wherein the roasted coffee beans have a reduced vinyl-guiacol content of less than about 100 mg/kg roasted coffee beans, and a reduced ethyl-pyrazine content of less than about 10 mg/kg roasted coffee beans. 32. A method for preparing Robusta or Arabica quality coffee beans having improved coffee flavor, said method comprising: (1) extracting dry or pre-moistened Robusta or Arabica quality green coffee beans with an aqueous solution at about 60° C. to about 100° C. for about 2 to about 4 hours to obtain (i) an aqueous extract containing water-soluble flavor precursors at about 4 to about 40 weight percent soluble solids, and (ii) extracted wet coffee beans;(2) separating the aqueous extract and the extracted wet coffee beans;(3) treating the separated aqueous extract to modify the water-soluble flavor precursors to obtain modified water-soluble flavor precursors, wherein the modified water-soluble flavor precursors are contained in the treated separated aqueous extract or are soluble solids obtained from the treated separated aqueous extract, wherein the treating is selected from one of heating the separated aqueous extract to hydrolyze water-soluble flavor precursors to organic acids, reducing levels of coumaryltryptophan and caffeoyltryptophan in the separated aqueous extract by contacting the separated aqueous extract with a hydrophobic or cation exchange resin, and treating the separated aqueous extract with a microorganism to reduce levels of caffeoylquinic acid and feruloylquinic acid in the separated extract;(4) combining the modified water-soluble flavor precursors with the separated extracted wet coffee beans before drying to provide flavor-enhanced coffee beans; and(5) drying the flavor-enhanced coffee beans to obtain the Robusta or Arabica quality coffee beans having improved coffee flavor,wherein the aqueous solution used in step (1) comprises previously treated extract from step (3) which is recycled to step (1) whereby the previously treated extract replaces one or more constituents in the dry or pre-moistened Robusta or Arabica quality green coffee beans.
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