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Science, v.291 no.5506 = no.5506, 2001년, pp.1021 - 1023
Chen, Banglin (Department of Chemistry, University of Michigan, Ann Arbor, MI 48109, USA.) , Eddaoudi, M. (Department of Chemistry, University of Michigan, Ann Arbor, MI 48109, USA.) , Hyde, S. T. (Department of Applied Mathematics, Australian National University, Canberra, Australia.) , O'Keeffe, M. (Department of Chemistry, Arizona State University, Tempe, AZ 85287, USA.) , Yaghi, O. M. (Department of Chemistry, University of Michigan, Ann Arbor, MI 48109, USA.)
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Interpenetration (catenation) has long been considered a major impediment in the achievement of stable and porous crystalline structures. A strategy for the design of highly porous and structurally stable networks makes use of metal-organic building blocks that can be assembled on a triply periodic...
10.1002/9783527613724 J. P. Sauvage C. Dietrich-Buchecker Eds. Molecular Catenanes Rotaxanes and Knots (Wiley-VCH New York 1999).
Raymo, F. M., Stoddart, J. F.. Interlocked Macromolecules. Chemical reviews, vol.99, no.7, 1643-1664.
Seeman, Nadrian C.. DNA NANOTECHNOLOGY: Novel DNA Constructions. Annual review of biophysics and biomolecular structure, vol.27, 225-248.
Storhoff, J. J., Mirkin, C. A.. Programmed Materials Synthesis with DNA. Chemical reviews, vol.99, no.7, 1849-1862.
Wikoff, William R., Liljas, Lars, Duda, Robert L., Tsuruta, Hiro, Hendrix, Roger W., Johnson, John E.. Topologically Linked Protein Rings in the Bacteriophage HK97 Capsid. Science, vol.289, no.5487, 2129-2133.
10.1002/(SICI)1521-3773(19980619)37:11<1460::AID-ANIE1460>3.0.CO;2-Z
For the design of intergrown nets with optimal porosity see T. M. Reineke M. Eddaoudi D. Moler M. O'Keeffe
Reineke, T. M., Eddaoudi, M., Moler, D., O'Keeffe, M., Yaghi, O. M.. Large Free Volume in Maximally Interpenetrating Networks: The Role of Secondary Building Units Exemplified by Tb2(ADB)3[(CH3)2SO]4·16[(CH3)2SO]1. Journal of the American Chemical Society, vol.122, no.19, 4843-4844.
M. O'Keeffe
O'Keeffe, M., Eddaoudi, M., Li, H., Reineke, T., Yaghi, O.M.. Frameworks for Extended Solids: Geometrical Design Principles. Journal of solid state chemistry, vol.152, no.1, 3-20.
M. O'Keeffe B. G. Hyde Crystal Structures I: Patterns and Symmetry (Mineralogical Society of America Washington DC 1996).
S. T. Hyde et al. The Language of Shape (Elsevier Amsterdam 1997).
The vertices of two interpenetrating diamond nets form the dense body-centered cubic array as in the structures of NaTl compounds [see e.g. (8)].
For a recent example and references see
Chen, B., Eddaoudi, M., Reineke, T. M., Kampf, J. W., O'Keeffe, M., Yaghi, O. M.. Cu2(ATC)·6H2O: Design of Open Metal Sites in Porous Metal−Organic Crystals (ATC: 1,3,5,7-Adamantane Tetracarboxylate). Journal of the American Chemical Society, vol.122, no.46, 11559-11560.
Details of the elemental analysis and crystal structures for as-synthesized and evacuated MOF-14 [ Im 3 a = 26.946(2) and 26.919(1) Å respectively] and the elemental analysis of solvent-exchanged MOF-14 are available at Science Online (www.sciencemag.org/cgi/content/full/291/5506/1021/DC1). X-ray coordinates have been deposited with the Cambridge Data Bank.
Weber, Edwin, Hecker, Manfred, Koepp, Erich, Orlia, Wolfgang, Czugler, Mátyás, Csöregh, Ingeborg. New trigonal lattice hosts: stoicheiometric crystal inclusions of laterally trisubstituted benzenes—X-ray crystal structure of 1,3,5-tris-(4-carboxyphenyl)benzene·dimethylformamide. Journal of the Chemical Society. Perkin transactions 2, vol.1988, no.7, 1251-1257.
H. Li M. Eddaoudi M. O'Keeffe
Li, Hailian, Eddaoudi, Mohamed, O'Keeffe, M., Yaghi, O. M.. Design and synthesis of an exceptionally stable and highly porous metal-organic framework. Nature, vol.402, no.6759, 276-279.
Eddaoudi, M., Li, H., Yaghi, O. M.. Highly Porous and Stable Metal−Organic Frameworks: Structure Design and Sorption Properties. Journal of the American Chemical Society, vol.122, no.7, 1391-1397.
D. W. Breck Zeolite Molecular Sieves (Wiley New York 1974).
Supported by NSF grants DMR-9804817 (M.O'K.) and CHE-9980469 (O.M.Y.) and by the U.S. Department of Energy (O.M.Y.). We thank S. Ramsden for production of Fig. 2.
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