[논문]Side Chain Engineered Naphthalene Diimide-Based Terpolymer for Efficient and Mechanically Robust All-Polymer Solar Cells

Lee, Jin-Woo; Choi, Nayoun; Kim, Dongjun; Phan, Tan Ngoc-Lan; Kang, Hyunbum; Kim, Taek-Soo; Kim, Bumjoon J.

doi:10.1021/acs.chemmater.0c04721

[해외논문] Side Chain Engineered Naphthalene Diimide-Based Terpolymer for Efficient and Mechanically Robust All-Polymer Solar Cells

Chemistry of materials : a publication of the American Chemical Society, v.33 no.3, 2021년, pp.1070 - 1081

Lee, Jin-Woo , Choi, Nayoun , Kim, Dongjun , Phan, Tan Ngoc-Lan , Kang, Hyunbum , Kim, Taek-Soo , Kim, Bumjoon J.

Abstract ▼ AI-Helper

The recent evolution of new polymer acceptors (PAs) using small-molecule building blocks with high light absorption has significantly increased the power conversion efficiency (PCE) of all-polymer solar cells (all-PSCs), but their mechanical properties are typically poor. Thus, poly[[N,N′-bis(2-octyldodecyl)-naphthalene-1,4,5,8-bis(dicarboximide)-2,6-diyl]-alt-5,5′-(2,2′-bithiophene)] (N2200) is still considered one of the most successful PAs in all-PSCs. Herein, we report the development of new naphthalene dimide-based PAs (NDI-PAs) that enable the achievement of both superior PCEs and mechanical robustness of all-PSCs compared to those of N2200-based devices. Our approach is very simple and effective for constructing a series of PAs [PNDIHD/DT-x, where x = 0-1], consisting of two NDI units with different side chains (2-hexyldecyl (HD) and 2-decyltetradecyl (DT)). The PNDIHD/DT-0.41-based all-PSCs with the poly[(2,6-(4,8-bis(5-(2-ethylhexyl)thiophen-2-yl)-benzo[1,2-b:4,5-b′]dithiophene))-alt-(5,5-(1′,3′-di-2-thienyl-5′,7′-bis(2-ethylhexyl)benzo[1′,2′-c:4′,5′-c′]dithiophene-4,8-dione))] (PBDB-T) polymer donor achieve a PCE of 9.3%, which outperforms the N2200-based device (PCE = 7.7%). This is mainly attributed to the enhanced charge generation and transport abilities of the PNDIHD/DT-0.41-based all-PSCs, as a result of optimal domain size and purity as well as high electron mobility. Importantly, the PBDB-T:PNDIHD/DT-0.41 blend shows excellent mechanical robustness, with a crack onset strain (COS) of 30% and a toughness of 7.5 MJ m-3. In addition, a flexible polymer solar cell (FPSC) device with the PBDB-T:PNDIHD/DT-0.41 blend shows a high initial PCE of 6.73%, which is maintained over 6% even after bending 1500 times.[FIG OMISSION]

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Armin, Ardalan, Kassal, Ivan, Shaw, Paul E., Hambsch, Mike, Stolterfoht, Martin, Lyons, Dani M., Li, Jun, Shi, Zugui, Burn, Paul L., Meredith, Paul. Spectral Dependence of the Internal Quantum Efficiency of Organic Solar Cells: Effect of Charge Generation Pathways. Journal of the American Chemical Society, vol.136, no.32, 11465-11472.

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Blom, P. W. M., Mihailetchi, V. D., Koster, L. J. A., Markov, D. E.. Device Physics of Polymer:Fullerene Bulk Heterojunction Solar Cells. Advanced materials, vol.19, no.12, 1551-1566.

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Koster, L. J. A., Mihailetchi, V. D., Xie, H., Blom, P. W. M.. Origin of the light intensity dependence of the short-circuit current of polymer/fullerene solar cells. Applied physics letters, vol.87, no.20, 203502-.

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Cowan, Sarah R., Roy, Anshuman, Heeger, Alan J.. Recombination in polymer-fullerene bulk heterojunction solar cells. Physical review. B, Condensed matter and materials physics, vol.82, no.24, 245207-.

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Hahn, Tobias, Tscheuschner, Steffen, Kahle, Frank‐Julian, Reichenberger, Markus, Athanasopoulos, Stavros, Saller, Christina, Bazan, Guillermo C., Nguyen, Thuc‐Quyen, Strohriegl, Peter, Bässler, Heinz, Köhler, Anna. Monomolecular and Bimolecular Recombination of Electron–Hole Pairs at the Interface of a Bilayer Organic Solar Cell. Advanced functional materials, vol.27, no.1, 1604906-.

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Kim, Hong Il, Kim, Minjun, Park, Cheol Woong, Kim, Hae Un, Lee, Han-Koo, Park, Taiho. Morphological Control of Donor/Acceptor Interfaces in All-Polymer Solar Cells Using a Pentafluorobenzene-Based Additive. Chemistry of materials : a publication of the American Chemical Society, vol.29, no.16, 6793-6798.

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Kotlarski, Jan D., Moet, Date J. D., Blom, Paul W. M.. Role of balanced charge carrier transport in low band gap polymer:Fullerene bulk heterojunction solar cells. Journal of polymer science Part B, Polymer physics, vol.49, no.10, 708-711.

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Zhang, Yannan, Xu, Yalong, Ford, Michael J., Li, Fangchao, Sun, Jianxia, Ling, Xufeng, Wang, Yongjie, Gu, Jinan, Yuan, Jianyu, Ma, Wanli. Thermally Stable All‐Polymer Solar Cells with High Tolerance on Blend Ratios. Advanced energy materials, vol.8, no.18, 1800029-.

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Li, Weiwei, Hendriks, Koen H., Furlan, Alice, Roelofs, W. S. C., Meskers, Stefan C. J., Wienk, Martijn M., Janssen, René A. J.. Effect of the Fibrillar Microstructure on the Efficiency of High Molecular Weight Diketopyrrolopyrrole‐Based Polymer Solar Cells. Advanced materials, vol.26, no.10, 1565-1570.

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Pang, Shuting, Zhang, Ruiwen, Duan, Chunhui, Zhang, Song, Gu, Xiaodan, Liu, Xi, Huang, Fei, Cao, Yong. Alkyl Chain Length Effects of Polymer Donors on the Morphology and Device Performance of Polymer Solar Cells with Different Acceptors. Advanced energy materials, vol.9, no.30, 1901740-.

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Mukherjee, Subhrangsu, Proctor, Christopher M., Tumbleston, John R., Bazan, Guillermo C., Nguyen, Thuc‐Quyen, Ade, Harald. Importance of Domain Purity and Molecular Packing in Efficient Solution‐Processed Small‐Molecule Solar Cells. Advanced materials, vol.27, no.6, 1105-1111.

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Lee, Changyeon, Giridhar, Thota, Choi, Joonhyeong, Kim, Seonha, Kim, Youngwoong, Kim, Taesu, Lee, Wonho, Cho, Han-Hee, Wang, Cheng, Ade, Harald, Kim, Bumjoon J.. Importance of 2D Conjugated Side Chains of Benzodithiophene-Based Polymers in Controlling Polymer Packing, Interfacial Ordering, and Composition Variations of All-Polymer Solar Cells. Chemistry of materials : a publication of the American Chemical Society, vol.29, no.21, 9407-9415.

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Lee, Jin‐Woo, Sun, Cheng, Ma, Boo Soo, Kim, Hyeong Jun, Wang, Cheng, Ryu, Jong Min, Lim, Chulhee, Kim, Taek‐Soo, Kim, Yun‐Hi, Kwon, Soon‐Ki, Kim, Bumjoon J.. Efficient, Thermally Stable, and Mechanically Robust All‐Polymer Solar Cells Consisting of the Same Benzodithiophene Unit‐Based Polymer Acceptor and Donor with High Molecular Compatibility. Advanced energy materials, vol.11, no.5, 2003367-.

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