[논문]Bioinspired nacre-like alumina with a bulk-metallic glass-forming alloy as a compliant phase

Wat, Amy; Lee, Je In; Ryu, Chae Woo; Gludovatz, Bernd; Kim, Jinyeon; Tomsia, Antoni P.; Ishikawa, Takehiko; Schmitz, Julianna; Meyer, Andreas; Alfreider, Markus; Kiener, Daniel; Park, Eun Soo; Ritchie, Robert O.

doi:10.1038/s41467-019-08753-6

[해외논문] Bioinspired nacre-like alumina with a bulk-metallic glass-forming alloy as a compliant phase 원문보기

Nature communications, v.10 no.1, 2019년, pp.961 -

Wat, Amy (Department of Materials Science and Engineering, University of California, Berkeley, CA 94720 USA) , Lee, Je In (Research Institute of Advanced Materials, Department of Materials Science and Engineering, Seoul National University, Seoul, 08826 Republic of Korea) , Ryu, Chae Woo (Research Institute of Advanced Materials, Department of Materials Science and Engineering, Seoul National University, Seoul, 08826 Republic of Korea) , Gludovatz, Bernd (School of Mechanical and Manufacturing Engineering, UNSW Sydney, Sydney, NSW 2052 Australia) , Kim, Jinyeon (Research Institute of Advanced Materials, Department of Materials Science and Engineering, Seoul National University, Seoul, 08826 Republic of Korea) , Tomsia, Antoni P. (Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720 USA) , Ishikawa, Takehiko (Japan Aerospace Explanation Agency, 2-1-1 Sengen, Tsukuba, Ibaraki 305-8505 Japan) , Schmitz, Julianna (Institut fü) , Meyer, Andreas (r Materialphysik im Weltraum, DLR, Kö) , Alfreider, Markus (ln, 51170 Germany) , Kiener, Daniel (Institut fü) , Park, Eun Soo (r Materialphysik im Weltraum, DLR, Kö) , Ritchie, Robert O. (ln, 51170 Germany)

Abstract ▼ AI-Helper

Bioinspired ceramics with micron-scale ceramic “bricks” bonded by a metallic “mortar” are projected to result in higher strength and toughness ceramics, but their processing is challenging as metals do not typically wet ceramics. To resolve this issue, we made alumina structures using rapid pressureless infiltration of a zirconium-based bulk-metallic glass mortar that reactively wets the surface of freeze-cast alumina preforms. The mechanical properties of the resulting Al2O3 with a glass-forming compliant-phase change with infiltration temperature and ceramic content, leading to a trade-off between flexural strength (varying from 89 to 800 MPa) and fracture toughness (varying from 4 to more than 9 MPa·m½). The high toughness levels are attributed to brick pull-out and crack deflection along the ceramic/metal interfaces. Since these mechanisms are enabled by interfacial failure rather than failure within the metallic mortar, the potential for optimizing these bioinspired materials for damage tolerance has still not been fully realized.Producing nacre-like ceramics with a tough, non-polymeric matrix remains a challenge. Here, the authors use the reactive wetting of a zirconium-based bulk metallic glass to successfully infiltrate a porous alumina and create a composite with improved flexural strength and fracture toughness.

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