[논문]Boosting electrostriction and strain performance in bismuth sodium titanate-based ceramics via introducing low tolerance factor chemical modifier

Ullah Khan, Naimat; Ullah, Aman; Ullah, Amir; Khan, Muhammad Yaqoob; Kim, Tae Heon; Kim, Ill Won; Ahn, Chang Won

doi:10.1016/j.sna.2019.03.043

[해외논문] Boosting electrostriction and strain performance in bismuth sodium titanate-based ceramics via introducing low tolerance factor chemical modifier

Sensors and actuators. A, Physical, v.291, 2019년, pp.156 - 166

Ullah Khan, Naimat (Department of Physics, University of Science & Technology) , Ullah, Aman (Department of Physics, University of Science & Technology) , Ullah, Amir (Department of Physics, Islamia College) , Khan, Muhammad Yaqoob (Department of Physics, Kohat University of Science & Technology) , Kim, Tae Heon (Department of Physics, University of Ulsan) , Kim, Ill Won (Department of Physics, University of Ulsan) , Ahn, Chang Won (Department of Physics, University of Ulsan)

Abstract ▼ AI-Helper

Abstract To realize giant electrostriction in BNT-based piezoelectrics, the tuning of thermotropic phase boundary (T F-R) towards ambient temperature is necessary. For the regulation of such T F-R, compositional modification approach either in the form of elemental doping or the substitution of higher tolerance factor ABO3 perovskite is usually preferred. In this study, we used a feasible approach to tune the T F-R of BNT-based system by introducing low tolerance factor ABO3 perovskite to achieve large strain response. To assess our synthetic approach, herein, a novel low tolerance factor perovskite Bi(Zn1/2Ce1/2)O3 is introduced as a chemical modifier and a ternary (0.935-x)Bi1/2Na1/2TiO3-0.065BaTiO3-xBi(Zn1/2,Ce1/2)O3 (BNT-BT-BZC) system is designed and prepared by solid state reaction method. By monitoring the temperature-dependent permittivity and tangent loss, a critical composition is detected for x = 0.015, at which the T F-R tuned down to room temperature (RT). By establishing the relationship between T F-R and electromechanical strain, the composition (x = 0.015) where T F-R situated below RT showed highest strain response (S = 0.43%) accompanied by a giant electrostrictive coefficient Q 33 ˜0.036 m4/C2. The derived Q 33 value is comparable to the prominent Pb-based counterparts and much higher than the reported lead-free BNT-based electrostrictors. Furthermore, favorable temperature stability in strain and electrostrictive performances is also demonstrated for the BNT-BT-BZC compound. We expect that our current work may provide a highly attractive way for the future development of lead-free electrostrictive materials. Highlights Giant electrostrictive coefficient Q 33 ˜0.036 m4/C2 was obtained in BNT-BT-BZC system. The derived Q 33 is comparable to Pb-based and higher than BNT-based electrostrictors. The electrostrictive coefficient shows favorable temperature stability up to 120 °C. BNT-BT-BZC system is promise for practical applications as lead-free electrostrictors. Graphical abstract [DISPLAY OMISSION]

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