[논문]Orientation Control of Semiconducting Polymers Using Microchannel Molds

Han, Moon Jong; Kim, Junkyu; Kim, Bomi; Park, Soon Mo; Ahn, Hyungju; Shin, Tae Joo; Kim, BongSoo; Kim, Hyoungsoo; Yoon, Dong Ki

doi:10.1021/acsnano.0c04138

[해외논문] Orientation Control of Semiconducting Polymers Using Microchannel Molds

ACS nano, v.14 no.10, 2020년, pp.12951 - 12961

Han, Moon Jong (Graduate School of Nanoscience and Technology , Korea Advanced Institute of Science and Technology , Daejeon , 34141 , Republic of Korea) , Kim, Junkyu (Department of Mechanical Engineering , Korea Advanced Institute of Science and Technology (KAIST) , Daejeon , 34141 , Republic of Korea) , Kim, Bomi (Department of Chemistry , Ulsan National Institute of Science and Technology (UNIST) , Ulsan , 44919 , Republic of Korea) , Park, Soon Mo (Graduate School of Nanoscience and Technology , Korea Advanced Institute of Science and Technology , Daejeon , 34141 , Republic of Korea) , Ahn, Hyungju (Pohang Accelerator Laboratory , Pohang , 37673 , Republic of Korea) , Shin, Tae Joo (UNIST Central Research Facilities , Ulsan National Institute of Science and Technology (UNIST) , Ulsan , 44919 , Republic of Korea) , Kim, BongSoo , Kim, Hyoungsoo , Yoon, Dong Ki

Abstract ▼ AI-Helper

The molecular orientation of organic semiconductors (OSCs) is of fundamental importance to anisotropic electrical behavior as well as superior properties in practical applications. Here, a simple and effective method is demonstrated to fabricate highly oriented semiconducting polymers, poly(3-hexylthiophene) (P3HT) and poly{[N,N′-bis(2-octyldodecyl)-1,4,5,8-naphthalenediimide-2,6-diyl]-alt-5,5′-(2,2′-bithiophene)} (P(NDI2OD-T2)), by mass transfer effect under microchannel molds by diffusion and convection. Furthermore, parallel or perpendicular molecular arrangements relative to the channel direction were achieved by varying the widths of the microchannels, which are directly observed using polarized optical microscopy and two-dimensional grazing-incidence X-ray diffraction experiments. The method could enable the fabrication of organic field-effect transistors that exhibit anisotropic electrical properties indicating inter- or intrachain charge transport. The resulting platform will provide a simple approach for multidirectional orientations of anisotropic OSCs.[FIG OMISSION]

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