[논문]Controlled Lattice Thermal Conductivity of Transparent Conductive Oxide Thin Film via Localized Vibration of Doping Atoms

Choi, Young Joong; Lee, Ho Yun; Kim, Seohan; Song, Pung Keun

doi:10.3390/nano11092363

Controlled Lattice Thermal Conductivity of Transparent Conductive Oxide Thin Film via Localized Vibration of Doping Atoms 원문보기

Nanomaterials, v.11 no.9, 2021년, pp.2363 -

Choi, Young Joong (Department of Materials Science and Engineering, Pusan National University, Busan 46241, Korea) , Lee, Ho Yun (yjchoi0782@pusan.ac.kr (Y.J.C.)) , Kim, Seohan (dbs0770@pusan.ac.kr (H.Y.L.)) , Song, Pung Keun (Department of Materials Science and Engineering, Pusan National University, Busan 46241, Korea)

Abstract ▼ AI-Helper

Amorphization using impurity doping is a promising approach to improve the thermoelectric properties of tin-doped indium oxide (ITO) thin films. However, an abnormal phenomenon has been observed where an excessive concentration of doped atoms increases the lattice thermal conductivity (κl). To elucidate this paradox, we propose two hypotheses: (1) metal hydroxide formation due to the low bond enthalpy energy of O and metal atoms and (2) localized vibration due to excessive impurity doping. To verify these hypotheses, we doped ZnO and CeO2, which have low and high bond enthalpies with oxygen, respectively, into the ITO thin film. Regardless of the bond enthalpy energy, the κl values of the two thin films increased due to excessive doping. Fourier transform infrared spectroscopy was conducted to determine the metal hydroxide formation. There was no significant difference in wave absorbance originating from the OH stretching vibration. Therefore, the increase in κl due to the excessive doping was due to the formation of localized regions in the thin film. These results could be valuable for various applications using other transparent conductive oxides and guide the control of the properties of thin films.

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참고문헌 (43)

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Controlled Lattice Thermal Conductivity of Transparent Conductive Oxide Thin Film via Localized Vibration of Doping Atoms 원문보기

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Controlled Lattice Thermal Conductivity of Transparent Conductive Oxide Thin Film via Localized Vibration of Doping Atoms 원문보기

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