[논문]Regular H-Bonding-Containing Polymers with Stretchability up to 100% External Strain for Self-Healable Plastic Transistors

Lee, Moo Yeol; Dharmapurikar, Satej; Lee, Sang Jin; Cho, Yongjoon; Yang, Changduk; Oh, Joon Hak

doi:10.1021/acs.chemmater.9b04574

[해외논문] Regular H-Bonding-Containing Polymers with Stretchability up to 100% External Strain for Self-Healable Plastic Transistors

Chemistry of materials : a publication of the American Chemical Society, v.32 no.5, 2020년, pp.1914 - 1924

Lee, Moo Yeol (School of Chemical and Biological Engineering, Institute of Chemical Processes , Seoul National University , 1 Gwanak-ro , Gwanak-gu, Seoul 08826 , South Korea) , Dharmapurikar, Satej (Department of Energy Engineering, School of Energy and Chemical Engineering, Perovtronics Research Center, Low Dimensional Carbon Materials Center , Ulsan National Institute of Science and Technology (UNIST) , 50 UNIST-gil , Ulsan 44919 , South Korea) , Lee, Sang Jin (Department of Chemical Engineering , Pohang University of Science and Technology (POSTECH) , 77 Cheongam-ro , Pohang 37673 , South Korea) , Cho, Yongjoon (Department of Energy Engineering, School of Energy and Chemical Engineering, Perovtronics Research Center, Low Dimensional Carbon Materials Center , Ulsan National Institute of Science and Technology (UNIST) , 50 UNIST-gil , Ulsan 44919 , South Korea) , Yang, Changduk , Oh, Joon Hak

Abstract ▼ AI-Helper

Intrinsically stretchable, electroactive materials featuring self-healing abilities will allow for a variety of next-generation stretchable electronics. Here, we synthesize diketopyrrolopyrrole-based “alternating” copolymers with urethane-containing side chains, that is, PDPPurethane copolymers, and use them as active layers in intrinsically stretchable and self-healable plastic transistors. The long-branched urethane side chains possessing moderate H-bonding strength enable sufficient solubility and excellent dynamic bonding, facilitating the stress dissipation under mechanical deformation. PDPPurethane thin films exhibit outstanding stretchability up to 100% external strain without degradation of electrical performance in the organic transistor platform. They also feature self-healing properties with the healing of cracks and the recovery of electrical properties after treatment. The structure-property relationships of PDPPurethane thin films under strain have been thoroughly investigated using a variety of characterization methods. Our results demonstrate a viable approach for the development of stretchable and self-healable plastic electronics using stretchable, semiconducting copolymers obtained via side chain engineering.[FIG OMISSION]

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