[논문]ZIF-8과 탄소기반물질 복합체를 이용한 슈퍼커패시터 및 화학센서의 최신연구동향

김상준; 이재민; 조승근; 이은빈; 이승기; 이정우

doi:10.5695/jsse.2022.55.2.51

ZIF-8과 탄소기반물질 복합체를 이용한 슈퍼커패시터 및 화학센서의 최신연구동향
Recent research trend of supercapacitor and chemical sensor using composite of ZIF-8 and carbon-based material 원문보기

한국표면공학회지 = Journal of the Korean institute of surface engineering, v.55 no.2, 2022년, pp.51 - 62

김상준 (부산대학교 재료공학부) , 이재민 (부산대학교 재료공학부) , 조승근 (부산대학교 재료공학부) , 이은빈 (부산대학교 재료공학부) , 이승기 (부산대학교 재료공학부) , 이정우 (부산대학교 재료공학부)

Abstract ▼ AI-Helper

Metal-organic framework (MOF) is one of the representative porous materials composed of metal ions and organic linkers. In spite of many advantages of the MOFs such as high specific surface area and ease of structure control, drawbacks have become obstacles to the practical use of them with poor electrical conductivity and chemical stability. The ZIF-8, which is consisted of zinc and imidazole linker, is one of the solutions to improve the chemical stability issue. In addition, composites using the ZIF-8 and carbonbased materials are widely used to enhance the electrical conductivity. In this regard, supercapacitor is very attractive field for using the composites, because most of carbon-based materials are porous and conductive. Also, for sensor applications, the ZIF-8 composite is suitable material to meet the requirement in terms of the selectivity and sensitivity. This review summarizes recent progress of the composite materials with the ZIF-8 and the carbon-based materials for the supercapacitors and the chemical sensors. In particular, the composites are classified into ZIF-8-graphene, ZIF-8-carbon nanotube and ZIF-8-other carbon-based material.

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그림 Fig. 1. Composite materials with the ZIF-8 and the carbon-based materials and its application.
표 Table. 1. Summary of composite materials with the ZIF-8 and the carbon-based materials for supercapacitors.
표 Table. 2. Summary of composite materials with the ZIF-8 and the carbon-based materials for chemical sensors.
그림 Fig. 2. (a) Fabrication of the graphene supported by hollow nitrogen-doped carbon frameworks. (b) CV curves of the GPNC at different scan rates. (c) CV of the GPNC, G/NC, and bulky NC. (d) GCD curves of the GPNC, G/NC, and bulky NC at 2 A g^-1. (e) The specific capacitances of the GPNC, G/NC, and bulky NC at different current densities, with permission of Chemistry Europe.
그림 Fig. 3. Schematic illustration for the preparation process of N-GQD@cZIF-8/CNT. (a) Heterogeneous nucleation of ZIF-8 onto CNTs. (b) Carbonization of ZIF-8/CNT and electrochemical deposition of N-GQDs on the cZIF-8/CNT matrix. (c) The evaluated optimum deposition condition of DC potential and electrodeposition time. (d) Cyclic voltammetry curves of cZIF-8, N-GQD@cZIF-8, cZIF-8/CNT, and N-GQD@cZIF- 8/CNT electrodes at a scan rate 10 mV s^-1 in 1.0 M H₂SO₄ electrolyte using a threeelectrode system, with permission of Wiley.
그림 Fig. 4. (a) Schematic illustration of the formation of the NCP-CNS composites. (b) CV curves of the NCP-CNS composites compared with NCPs and CNSs at 10 mV s^-1. (c) Specific capacitances of NCP-CNS composites compared with NCPs and CNSs calculated from the galvanostatic charge/discharge curves at different current densities. (d) CV curves of the NCPCNS-2 electrode at different scan rates. (e) Ragone plots for comparison of our supercapacitors with various ZIF-8 derived carbons and their composite materials previously reported, with permission of ACS publishing.
그림 Fig. 5. (a) Schematic of the modification step at the interface of the optical microfiber. Corresponding spectral shifts of (b) four-growth-cycles-ZIF-8/GO (orange dots) and (c) four-growth-cycles-ZIF-8 (purple dots) response to ethanol. The green dots represent the nonspecific spectral shifts response to methanol. (d) The spectral response to ethanol recorded by a bare optical microfiber, GO-functionalized optical microfiber, two-growth-cycles-ZIF-8/GOfunctionalized fiber, and four-growth-cycles-ZIF-8/GO-functionalized optical microfiber, with permission of Wiley.
그림 Fig. 6. (a) Schematic of the synthetic route of the C-dots/ZIF-8/MnO₂ and the AA detection process. (b) Selectivity of the probe for AA over other potential interferences (Na⁺: 1mM; K⁺: 0.5 mM; Mg²⁺ and Ca²⁺: 0.25 Mm; sodium citrate and glucose: 0.05 mM; sodium glutamate: 0.1 mM; soluble starch, DL-tartaric acid, glutathione, cysteine and bovine serum albumin: 10 μM; AA: 9 μM), F0 and F are the fluorescence intensity of the probe in the absence and presence of the target (AA) or nontarget samples, respectively, with permission of RSC publishing.

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