[논문]전고체 리튬 이차전지용 합금계 음극 소재의 연구 동향

윤정명; 박철민

doi:10.14773/cst.2023.22.6.466

전고체 리튬 이차전지용 합금계 음극 소재의 연구 동향
Recent Progress of Alloy-Based All-Solid-State Li-Ion Battery Anodes 원문보기

Corrosion science and technology, v.22 no.6, 2023년, pp.466 - 477

윤정명 (금오공과대학교 신소재공학과) , 박철민 (금오공과대학교 신소재공학과)

Abstract ▼ AI-Helper

The increasing demand for high-performance energy storage systems has highlighted the limitations of conventional Li-ion batteries (LIBs), particularly regarding safety and energy density. All-solid-state batteries (ASSBs) have emerged as a promising next-generation energy storage system, offering the potential to address these issues. By employing nonflammable solid electrolytes and utilizing high-capacity electrode materials, ASSBs have demonstrated improved safety and energy density. Automotive and energy storage industries, in particular, have recognized the significance of advancing ASSB technology. Although the use of Li metal as ASSB anode is promising due to its high theoretical capacity and the expectation that Li dendrites will not form in solid electrolytes, persistent problems with Li dendrite formation during cycling remain. Therefore, the exploration of novel high-performance anode materials for ASSBs is highly important. Recent research has focused extensively on alloy-based anodes for ASSBs, owing to their advantages of no dendrite formation and high-energy density. This study provides a comprehensive review of the latest advancements and challenges associated with alloy-based anodes for ASSBs.

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표/그림 (7)

그림 Fig. 1. Potential microstructural contributions to inhomogeneous Li plating from a solid electrolyte (SE) Left and middle; current focusing mechanisms resulting from poor interfacial wetting or fast Li-ion migration along grain boundaries; Right: accommodation of electrodeposited Li at soft grain boundaries [9] (Copyright 2018, American Chemical Society)
그림 Fig. 2. Electrochemical behavior of all-solid-state cells with aluminum-based negative electrodes a-e, Galvanostatic testing of Al and Al_94.5In_5.5 cells: (a) Al | LPSCl | NCM full cell voltage curves, (b) dQ/dV curves for the first two cycles of the Al-In, (c) Al_94.5In_5.5 | LPSCl | NCM full cell voltage curves, (d) dQ/dV curves comparing the first cycle of the Al to the Al-In cell, (e) Areal capacity with cycling, (f) Rate testing of Al | LPSCl | NCM and Al_94.5In_5.5 | LPSCl | NCM full cells, (g) GITT measurements of Al | LPSCl | Li (red) and Al_94.5In_5.5 | LPSCl | Li (blue) half cells with 10 MPa stack pressure;The open circles represent OCV values after the rest periods, and the solid lines are the voltage traces during current application; All testing was performed at 25 ℃ [29] (Copyright 2023, Springer Nature)
그림 Fig. 3. Electrochemical behavior of the different alloys Li stripping and plating performance of symmetrical A|Li₆ PS₅Cl|A (A = Li, Li_0.5In, LiIn, Li₁₃In₃) cells; (a) Li, (b) Li_0.5In, (c) LiIn, (d) Li₁₃In₃, the red dashed line in the polarization profiles corresponds to the overpotential (IR min) expected based on the resistance of the electrolyte pellet (RSE) and the interfacial resistance (R int), (e) Schematic illustration and comparison of the depletion mechanism for Li and the Li alloys, as well as the impedance elements used for the data interpretation, (f) Long-term Li cycling performance of the Li₁₃ In₃ |Li₆PS₅Cl|Li₁₃In₃ cell, (g) The corresponding Nyquist impedance profiles recorded before and after the cycling, (h) Computed Li⁺ migration energies in Li-In alloys [30] (Copyright 2021, American Chemical Society)
그림 Fig. 4. Characterization and electrochemical behavior of the Si/SE/CB composite anode; (a) Schematics of the preparation process of Si/SE/CB and the configuration of Si composite anode in ASLB, (b) SEM images of Si nanoparticles, (c) SEM images of Si/SE/CB, (d) Galvanostatic charge and discharge profiles, (e) Corresponding dQ/dV profiles of ASLB at the first cycle, (f) Rate performance of ASLB at current densities of 0.1, 0.2, 0.5, 1, and 2 mA cm^-2, (g) Long-term cycling performance of ASLB at a current density of 0.5 mA cm^-2 [26] (Copyright 2022, John Wiley and Sons)
그림 Fig. 5. Characterization and electrochemical behavior of the Sn/Graphite composite anode; (a) Schematics of the Sn/Graphite half-cell in ASSBs, b-c. Cross-sectional SEM images of anode composite in contact with SE, (b) before cycling, (c) after cycling, d-i Charge-discharge curves of (d) graphite and (e) Sn/Graphite-based electrodes, (f) Charge-discharge curves (2nd cycle) of Sn/ Graphite electrodes with various areal loadings, (g) Rate capability measurements of Sn/Graphite electrodes with the composition of 30:5:65 (Sn/Graphite/CNF/Li₃PS₄), (h) Cycle performance of Sn/Graphite and graphite, (i) Comparison of the selected voltage profiles of Sn/Graphite electrodes [46] (Copyright 2022, American Chemical Society)
그림 Fig. 6. Characterization and electrochemical behavior of the BP/NG/LiBH₄ composite anode; (a) Schematic illustration and HR-TEM image of C-P bond in BP/NG/LiBH₄ composite, (b) CV curves of BP/NG/LiBH₄ for initial four cycles in all-solidstate half-cell at a scan rate of 0.2 mV s^-1, (c) GDC curves and (d) rate performance of BP/NG/LiBH 4 composite at current densities from 0.2 A g^-1 to 1 A g^-1, (e) GDC curves of BP/NG/LiBH₄ for different cycles at the current density of 0.5 A g^-1 and (f) comparison of long cycling performance of BP/NG/LiBH₄, pure NG, and pure BP at the current density of 0.5 A g^-1 [50]
그림 Fig. 7. Characterization and electrochemical behavior of the GaSb/C/LiBH₄ composite anode; (a) Schematic illustration and Dynamic TEM image of GaSb/C/LiBH₄ electrode at 1.2 V, (b) GDC curves of GaSb/C/LiBH4 half cell at 1 A g^-1, (c) Corresponding cycle performance of GaSb/C/LiBH₄ half cell (d) GDC curves of GaSb/C/LiBH₄ |TiS₂ full cell at 1 A g^-1, (e) Corresponding cycle performance of GaSb/C/LiBH₄ |TiS₂ full cell [52] (Copyright 2020, American Chemical Society)

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표제어: PCR

동의어: Packet Collision Rate

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용어 설명: PCR은 세균 특이성이 있는 primer를 이용하여 적은 수의 세균이 있을지라도 쉽게 검출할 수 있는 유용한 방법이며, 이를 이용하여 구강 내 치면세균막이나 타액에서 직접 세균을 검출할 수 있게 되었다[8].

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저장형식	Text(ASCII format) Excel format RefWorks Direct Export RIS format (for Reference Manager, ProCite, EndNote), Scholar's Aids, Mendeley
메일정보	받는사람 (필수) @ 보내는사람 (선택) @ 제목 내용 KISTI 검색결과 이메일 서비스
안내	총 건의 자료가 검색되었습니다. 다운받으실 자료의 인덱스를 입력하세요. (1-10,000) 검색결과의 순서대로 최대 10,000건 까지 다운로드가 가능합니다. 데이타가 많을 경우 속도가 느려질 수 있습니다.(최대 2~3분 소요) 다운로드 파일은 UTF-8 형태로 저장됩니다. 파일의 내용이 제대로 보이지 않을실 때는 웹브라우저 상단의 보기 -> 인코딩 -> 자동선택 여부를 확인하십시오. ~ Text(ASCII format) Excel format

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